Chlorination: The CT Concept in Water Disinfection

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3.0-log inactivation — CT = 30 mg·min/L at pH 7, 15°C

At 1.0 mg/L free chlorine for 30 minutes (CT=30), pH 7, 15°C: achieves approximately 3.0-log inactivation of Giardia and 4+ log for viruses.

Formula

CT = C × t (mg·min/L)
Log inactivation = −log₁₀(N/N₀)
Chick-Watson: ln(N/N₀) = −k × C^n × t

The CT Framework

The CT (concentration × time) concept is the backbone of regulatory disinfection compliance worldwide. By multiplying the residual disinfectant concentration by the effective contact time, engineers get a single number that predicts pathogen inactivation. The USEPA Surface Water Treatment Rule specifies required CT values for different pathogens, temperatures, and pH levels — typically requiring 4-log virus and 3-log Giardia inactivation.

Chlorine Chemistry in Water

When chlorine gas or sodium hypochlorite is added to water, it forms hypochlorous acid (HOCl) and hypochlorite ion (OCl⁻). The equilibrium between these species depends on pH. HOCl is a small, neutral molecule that penetrates cell membranes far more effectively than the charged OCl⁻ ion. This pH dependence makes water chemistry control essential for reliable disinfection.

Temperature Effects

Disinfection kinetics follow Arrhenius-type temperature dependence. Colder water requires significantly higher CT values — roughly doubling for each 10°C decrease. This is why northern treatment plants in winter face the greatest disinfection challenges, often requiring higher chlorine doses or longer contact times that increase DBP formation potential.

Balancing Disinfection and Byproducts

The fundamental tension in chlorination is that the same chemical reaction that kills pathogens also creates potentially carcinogenic disinfection byproducts (DBPs). Treatment plants manage this by removing organic precursors before chlorination (enhanced coagulation, activated carbon), using alternative primary disinfectants (ozone, UV), and applying chlorine or chloramine as a secondary disinfectant for distribution system residual.

FAQ

What is the CT concept in water disinfection?

CT is the product of disinfectant Concentration (mg/L) and contact Time (minutes). It is the standard measure of disinfection dose. Different pathogens require different CT values for a given log inactivation — for example, 3-log Giardia inactivation requires CT ≈ 104 mg·min/L with free chlorine at pH 7, 15°C.

Why does pH affect chlorine disinfection?

Chlorine in water exists as hypochlorous acid (HOCl) and hypochlorite ion (OCl⁻). HOCl is 80-100× more effective as a disinfectant. At pH 7.5, they exist in roughly equal proportions. Above pH 8, OCl⁻ dominates, drastically reducing disinfection efficiency. This is why pH control is critical in treatment plants.

What are disinfection byproducts?

When chlorine reacts with natural organic matter in water, it forms trihalomethanes (THMs) and haloacetic acids (HAAs) — regulated carcinogens. Treatment plants must balance sufficient disinfection (high CT) against minimizing DBPs (low CT). This tension drives the use of alternative disinfectants like UV and ozone.

How much chlorine residual should drinking water have?

The USEPA requires a detectable chlorine residual (≥0.2 mg/L) entering the distribution system. Typical levels are 0.5-2.0 mg/L leaving the plant, declining through the pipe network. The residual provides ongoing protection against recontamination during distribution.

Sources

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