Leaching Kinetics Simulator: Shrinking-Core Model for Ore Dissolution

simulator intermediate ~10 min
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τ = 142 min — 95% copper extraction

A 2 mm ore particle in 1 mol/L H₂SO₄ at 50°C reaches 95% copper extraction in approximately 142 minutes, governed primarily by product-layer diffusion.

Formula

τ = ρ_B · R₀² / (6 · b · D_e · C_A) — diffusion-controlled complete reaction time
1 - 3(1-X)^(2/3) + 2(1-X) = t/τ — diffusion-controlled conversion
k(T) = A · exp(-E_a / RT) — Arrhenius temperature dependence

Dissolving the Ore

Leaching is the foundational step in hydrometallurgy: a solid ore particle is immersed in an acidic (or alkaline) solution that selectively dissolves the target metal. The shrinking-core model, developed by Yagi and Kunii in 1955 and refined by Levenspiel, provides an elegant mathematical framework for predicting how fast this dissolution proceeds. As the acid penetrates the particle surface, it reacts with the mineral, leaving behind a porous shell of gangue through which fresh acid must diffuse to reach the retreating reaction front.

Shrinking-Core Mathematics

The model distinguishes three sequential resistances: external film diffusion, product-layer diffusion, and surface chemical reaction. In most industrial settings, product-layer diffusion dominates for particles larger than ~1 mm. The key equation relates fractional conversion X to dimensionless time: 1 - 3(1-X)^(2/3) + 2(1-X) = t/τ, where τ is the time for complete conversion. This τ depends on particle radius squared, making size reduction the single most powerful lever for accelerating extraction.

Temperature and Activation Energy

The Arrhenius equation governs how temperature accelerates leaching. Diffusion-controlled processes have low activation energies (10–25 kJ/mol), while reaction-controlled processes show higher values (40–80 kJ/mol). This distinction is diagnostic: if doubling temperature barely changes the rate, diffusion controls. If the rate surges, chemical reaction is limiting. Industrial heap leaches operate at ambient temperature for cost reasons, while autoclave processes push to 150–250°C for refractory ores.

Industrial Applications

Heap leaching of copper oxides with sulfuric acid is one of the largest hydrometallurgical operations on Earth, processing billions of tonnes of ore annually in Chile, Peru, and Arizona. The same shrinking-core principles apply to pressure oxidation of gold ores, alkaline leaching of bauxite (Bayer process), and the emerging field of direct lithium extraction from brines. This simulator lets you explore how particle size, acid strength, and temperature interact to determine extraction efficiency and processing time.

FAQ

What is the shrinking-core model?

The shrinking-core model describes the dissolution of a solid particle from the outside inward. As leaching progresses, the unreacted core shrinks while a porous product layer (ash or gangue) grows around it. The model identifies three possible rate-limiting steps: fluid-film diffusion, product-layer diffusion, or chemical reaction at the core surface.

What controls leaching rate — diffusion or reaction?

For fine particles (<100 μm) and low temperatures, chemical reaction at the surface typically controls. For larger particles and higher temperatures, diffusion through the porous product layer dominates. Plotting 1-(1-X)^(1/3) vs time (reaction control) or 1-3(1-X)^(2/3)+2(1-X) vs time (diffusion control) reveals which mechanism fits.

How does particle size affect leaching time?

Leaching time scales with R₀² for diffusion-controlled processes and R₀ for reaction-controlled processes. This is why comminution (grinding) is one of the most impactful variables in hydrometallurgy — reducing particle size from 10 mm to 1 mm can reduce leaching time by 100×.

What acids are used in industrial leaching?

Sulfuric acid (H₂SO₄) is the workhorse for copper and zinc oxide ores. Hydrochloric acid is used for nickel laterites and rare earths. Cyanide solutions leach gold and silver. Alkaline leaching with NaOH dissolves alumina from bauxite in the Bayer process.

Sources

Embed

<iframe src="https://homo-deus.com/lab/hydrometallurgy/leaching-kinetics/embed" width="100%" height="400" frameborder="0"></iframe>
View source on GitHub